Harmonic Generation in Paramagnetic Spin Systems.
Abstract:
The theory of resonant second and third harmonic generation is considered and applied to the case of paramagnetic spin systems tuned by a magnetic field. Using available spectroscopic and material parameters, conversion efficiencies of around 25 seem feasible. Optical nonlinearities in semiconductor super-lattice are considered and shown to have large second order optical nonlinearities in the mid-infrared.
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