Accession Number:

AD1016744

Title:

Thermoelectric Transport in Surface- and Antimony-Doped Bismuth Telluride Nanoplates

Corporate Author:

University of Texas at Austin Austin United States

Report Date:

2016-07-25

Abstract:

We report the in-plane thermoelectric properties of suspended Bi1xSbx 2Te3nanoplates with x ranging from 0.07 to 0.95 and thicknesses ranging from 9 to42 nm. The results presented here reveal a trend of increasing p-type behavior with increasing antimony concentration, and a maximum Seebeck coefficient and thermoelectric figure of merit at x 0.5. We additionally tuned extrinsic doping of the surface using a tetrafluoro-tetracyanoquinodimethane F4-TCNQ coating. The lattice thermal conductivity is found to be below that for undoped ultrathin Bi2Te3 nanoplates of comparable thickness and in the range of 0.20.7 W m1 K1at room temperature.

Descriptive Note:

Journal Article

Supplementary Note:

APL Materials , 4, 10, 01 Jan 0001, 01 Jan 0001, Open Access: Publishers Version. May be placed on public websites; Creative Commons Attribution (CC BY) license (http://creativecommons.org/licenses/by/4.0/)

Pages:

0009

Communities Of Interest:

Modernization Areas:

Distribution Statement:

Approved For Public Release;

File Size:

2.74MB