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Enabling Remote Quantum Emission in 2d Semiconductors Via Porous Metallic Networks

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Journal Article - Open Access

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Naval Research Lab Washington United States

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Here we report how two-dimensional crystal 2DC overlayers influence the recrystallization of relatively thick metal films and the subsequent synergetic benefits this provides for coupling surface plasmon-polaritons SPPs to photon emission in 2D semiconductors. We show that annealing 2DCAu films on SiO2 results in a reverse epitaxial process where initially nanocrystalline Au films gain texture, crystallographically orient with the 2D crystal overlayer, and form an oriented porous metallic network OPEN structure in which the 2DC can suspend above or coat the inside of the metal pores. Both laser excitation and exciton recombination in the 2DC semiconductor launch propagating SPPs in the OPEN film. Energy in-out- coupling occurs at metal pore sites, alleviating the need for dielectric spacers between the metal and 2DC layer. At low temperatures, single-photon emitters SPEs are present across an OPEN-WSe2 film, and we demonstrate remote SPP-mediated excitation of SPEs at a distance of 17 mu m.

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  • Crystallography

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